Latest News

Here you find current and previous news from the PSI Center for Neutron and Muon Sciences. 

Understanding the Enhanced Magnetic Response of Aminocholesterol Doped Lanthanide-Ion-Chelating Phospholipid Bicelles

Cholesterol (Chol-OH) and its conjugates are powerful molecules for engineering the physicochemical and magnetic properties of phospholipid bilayers in bicelles.

Three-dimensional magnetization structures revealed with X-ray vector nanotomography

In soft ferromagnetic materials, the smoothly varying magnetization leads to the formation of fundamental patterns such as domains, vortices and domain walls. These have been studied extensively in thin films of thicknesses up to around 200 nanometres, in which the magnetization is accessible with current transmission imaging methods that make use of electrons or soft X-rays.

The neutron spectrometer TASP used in this study ©PSI

New quantum state observed in a Shastry–Sutherland compound

Scientists from PSI and the École polytechnique fédérale de Lausanne (EPFL) have shown experimentally, for the first time, a quantum phase transition in strontium copper borate, the only material to date that realizes the famous Shastry–Sutherland quantum many-body model.

4-spin plaquette singlet state in the Shastry–Sutherland compound SrCu2(BO3)2

The study of interacting spin systems is of fundamental importance for modern condensed-matter physics. On frustrated lattices, magnetic exchange interactions cannot be simultaneously satisfied, and often give rise to competing exotic ground states. The frustrated two-dimensional Shastry–Sutherland lattice realized by SrCu2(BO3)2 is an important test to our understanding of quantum magnetism.

Three-Dimensional Electronic Structure of the Type-II Weyl Semimetal WTe2

By combining bulk sensitive soft-x-ray angular-resolved photoemission spectroscopy and first- principles calculations we explored the bulk electron states of WTe2, a candidate type-II Weyl semimetal featuring a large nonsaturating magnetoresistance. Despite the layered geometry suggesting a two-dimensional electronic structure, we directly observe a three-dimensional electronic dispersion.

Quantum Griffiths Phase Inside the Ferromagnetic Phase of Ni1-xVx

We study by means of bulk and local probes the d-metal alloy Ni1-xVx close to the quantum critical concentration, xc ≈ 11.6%, where the ferromagnetic transition temperature vanishes. The magnetization-field curve in the ferromagnetic phase takes an anomalous power-law form with a nonuniversal exponent that is strongly x dependent and mirrors the behavior in the paramagnetic phase.

Comparison of ultracold neutron sources for fundamental physics measurements

Ultracold neutrons (UCNs) are key for precision studies of fundamental parameters of the neutron and in searches for new charge-parity-violating processes or exotic interactions beyond the Standard Model of particle physics. The most prominent example is the search for a permanent electric-dipole moment of the neutron (nEDM). We have performed an experimental comparison of the leading UCN sources currently operating.

Methods for Generating Highly Magnetically Responsive Lanthanide-Chelating Phospholipid Polymolecular Assemblies

Mixtures of 1,2-dimyristoyl-sn-glycero-3-phosphocholine (DMPC) and its lanthanide ion (Ln3+) chelating phospholipid conjugate, 1,2-dimyristoyl-sn-glycero-3-phospho-ethanolamine-diethylene triaminepentaacetate (DMPE-DTPA), assemble into highly magnetically responsive polymolecular assemblies such as DMPC/DMPE-DTPA/Ln3+ (molar ratio 4:1:1) bicelles.

Superlattice growth and rearrangement during evaporation-induced nanoparticle self-assembly

Understanding the assembly of nanoparticles into superlattices with well-defined morphology and structure is technologically important but challenging as it requires novel combinations of in-situ methods with suitable spatial and temporal resolution.

Coupled multiferroic domain switching in the canted conical spin spiral system Mn2GeO4

Despite remarkable progress in developing multifunctional materials, spin-driven ferro-electrics featuring both spontaneous magnetization and electric polarization are still rare. Among such ferromagnetic ferroelectrics are conical spin spiral magnets with a simultaneous reversal of magnetization and electric polarization that is still little understood. Such materials can feature various multiferroic domains that complicates their study.

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Distinct, but not so different

Among superconducting materials, CeCoIn5 stands out as a rare case where superconductivity gives rise to magnetic order. An international team led by PSI physicist Michel Kenzelmann now reports that when small amounts of impurities are implanted into CeCoIn5, then two distinct magnetic phases appear — and these are surprisingly similar to one another.

Pressure-induced magnetic order in FeSe: A muon spin rotation study

The magnetic order induced by the pressure was studied in FeSe by means of muon spin rotation (μSR) technique.

Emergent magnetism at transition-metal-nanocarbon interfaces

Interfaces are critical in quantum physics, and therefore we must explore the potential for designer hybrid materials that profit from promising combinatory effects. In particular, the fine-tuning of spin polarization at metallo–organic interfaces opens a realm of possibilities, from the direct applications in molecular spintronics and thin-film magnetism to biomedical imaging or quantum computing.

Determination of Conduction and Valence Band Electronic Structure of LaTiOxNy Thin Films

The nitrogen substitution into the oxygen sites of several oxide materials leads to a reduction of the band gap to the visible-light energy range, which makes these oxynitride semiconductors potential photocatalysts for efficient solar water splitting. Oxynitrides typically show a different crystal structure compared to the pristine oxide material.

Unconventional magnetic order in the conical state of MnSi

In the temperature-magnetic field phase diagram, the binary metallic compound MnSi exhibits three magnetic phases below Tc ≈ 29K.An unconventional helicoidal phase is observed in zero field. At moderate field intensity a conical phase sets in. Near Tc, in an intermediate field range, a skyrmion lattice phase appears.

Anomalous Thermal Conductivity and Magnetic Torque Response in the Honeycomb Magnet α-RuCl3

We report on the unusual behavior of the in-plane thermal conductivity κ and torque τ response in the Kitaev-Heisenberg material α-RuCl3. κ shows a striking enhancement with linear growth beyond H = 7T, where magnetic order disappears, while τ for both of the in-plane symmetry directions shows an anomaly at the same field.

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Climbing the ladder

Quantum phenomena can lead to intriguing effects in materials, but are famously difficult to predict and understand. A combined experimental and theoretical study of a model quantum system provides insight into excitations that involve multiple particles at once.

Bound States and Field-Polarized Haldane Modes in a Quantum Spin Ladder

The challenge of one-dimensional systems is to understand their physics beyond the level of known elementary excitations. By high-resolution neutron spectroscopy in a quantum spin-ladder material, we probe the leading multiparticle excitation by characterizing the two-magnon bound state at zero field.

Amyloid fibril systems reduce, stabilize and deliver bioavailable nanosized iron

Iron-deficiency anaemia (IDA) is a major global public health problem. A sustainable and cost-effective strategy to reduce IDA is iron fortification of foods, but the most bioavailable fortificants cause adverse organoleptic changes in foods. Iron nanoparticles are a promising solution in food matrices, although their tendency to oxidize and rapidly aggregate in solution severely limits their use in fortification.

Doping Dependence of Collective Spin and Orbital Excitations in the Spin-1 Quantum Antiferromagnet La2-xSrxNiO4 Observed by X-Rays

We report the first empirical demonstration that resonant inelastic x-ray scattering (RIXS) is sensitive to collective magnetic excitations in S=1 systems by probing the Ni L3 edge of La2-xSrxNiO4 (x=0, 0.33, 0.45). The magnetic excitation peak is asymmetric, indicating the presence of single and multi-spin-flip excitations.

Amplitude Mode in Three-Dimensional Dimerized Antiferromagnets

The amplitude ("Higgs") mode is a ubiquitous collective excitation related to spontaneous breaking of a continuous symmetry. We combine quantum Monte Carlo (QMC) simulations with stochastic analytic continuation to investigate the dynamics of the amplitude mode in a three-dimensional dimerized quantum spin system.

High hydrostatic pressure specifically affects molecular dynamics and shape of low-density lipoprotein particles

Lipid composition of human low-density lipoprotein (LDL) and its physicochemical characteristics are relevant for proper functioning of lipid transport in the blood circulation. To explore dynamical and structural features of LDL particles with either a normal or a triglyceride-rich lipid composition we combined coherent and incoherent neutron scattering methods.

LaTiOxNy thin film model systems for photocatalytic water splitting: physicochemical evolution of the solid-liquid interface and the role of the crystallographic orientation

The size of the band gap and the energy position of the band edges make several oxynitride semiconductors promising candidates for efficient hydrogen and oxygen production under solar light illumination. The intense research efforts dedicated to oxynitride materials have unveiled the majority of their most important properties. However, two crucial aspects have received much less attention.

Gapless Spin-Liquid Ground State in the S=1/2 Kagome Antiferromagnet

The defining problem in frustrated quantum magnetism, the ground state of the nearest-neighbor S=1/2 antiferromagnetic Heisenberg model on the kagome lattice, has defied all theoretical and numerical methods employed to date. We apply the formalism of tensor-network states, specifically the method of projected entangled simplex states, which combines infinite system size with a correct accounting for multipartite entanglement.

Magnetic states of MnP: muon-spin rotation studies

Muon-spin rotation data collected at ambient pressure (p) and at p = 2.42 GPa in MnP were analyzed to check their consistency with various low- and high-pressure magnetic structures reported in the literature. Our analysis con rms that in MnP the low-temperature and low-pressure helimagnetic phase is characterised by an increased value of the average magnetic moment compared to the high-temperature ferromagnetic phase.

Tuning the multiferroic mechanisms of TbMnO3 by epitaxial strain

A current challenge in the field of magnetoelectric multiferroics is to identify systems that allow a controlled tuning of states displaying distinct magnetoelectric responses. Here we show that the multiferroic ground state of the archetypal multiferroic TbMnO3 is dramatically modified by epitaxial strain. Neutron diffraction reveals that in highly strained films the magnetic order changes from the bulk-like incommensurate bc-cycloidal structure to commensurate magnetic order.

Sub-pixel correlation length neutron imaging: Spatially resolved scattering information of microstructures on a macroscopic scale

Neutron imaging and scattering give data of significantly different nature and traditional methods leave a gap of accessible structure sizes at around 10 micrometers. Only in recent years overlap in the probed size ranges could be achieved by independent application of high resolution scattering and imaging methods, however without providing full structural information when microstructures vary on a macroscopic scale.

High-resolution non-destructive three-dimensional imaging of integrated circuits

Modern nanoelectronics has advanced to a point at which it is impossible to image entire devices and their interconnections non- destructively because of their small feature sizes and the complex three-dimensional structures resulting from their integration on a chip. This metrology gap implies a lack of direct feedback between design and manufacturing processes, and hampers quality control during production, shipment and use.

Ground state selection under pressure in the quantum pyrochlore magnet Yb2Ti2O7

A quantum spin liquid is a state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho2Ti2O7 and Dy2Ti2O7, so-called spin ices, exhibit a classical spin liquid state with fractionalized thermal excitations (magnetic monopoles).