LNS - Scientific Highlights

The anomalous Hall effect (AHE) has emerged as a key indicator of time-reversal symmetry breaking (TRSB) and topological features in electronic band structures. Absent of a magnetic field, the AHE requires spontaneous TRSB but has proven hard to probe due to averaging over domains. The anomalous component of the Hall effect is thus frequently derived from extrapolating the magnetic field dependence of the Hall response. We show ....

Multiband superconductivity arises when multiple electronic bands contribute to the formation of the superconducting state, allowing distinct pairing interactions and gap structures. Here, we present field- and temperature-dependent data  ...

The spiral spin liquid (SSL) is a highly degenerate state characterized by a continuous contour or surface in reciprocal space spanned by a spiral propagation vector. Although the SSL state has been predicted in a number of various theoretical models, very few materials are so far experimentally identified to host such a state. Via combined single-crystal wide-angle and small-angle neutron scattering, we report observation  ...

Encoding information in antiferromagnetic (AFM) domains is a promising solution for the ever growing demand in magnetic storage capacity. The absence of a macroscopic magnetization avoids crosstalk between different domain states, enabling ultrahigh density spintronics while being detrimental to the domain detection and manipulation. Disentangling these merits and disadvantages seemed so far unattainable. We report evidence ...

Spin moiré superlattices (SMSs) formed by interfacing conventional electronic states with a multi-q magnetic lattice have been proposed as a magnetic analog of crystallographic moiré systems. The electron-minibands created in an SMS are expected to be enriched by the vector-field nature of the magnetic interaction and offer new types of moiré tunability, topological protection, and Berry curvature effects. However, most spin-vortex-hosting systems discovered to date have carrier mean free paths l_mfp significantly shorter than their spin-moiré lattice constant a_spin, inhibiting mini-band-formation. Furthermore ...

Skyrmions are particlelike vortices of magnetization with nontrivial topology, which are usually stabilized by Dzyaloshinskii-Moriya interactions (DMI) in noncentrosymmetric bulk materials. Exceptions are centrosymmetric Gd- and Eu-based skyrmion-lattice (SL) hosts with zero DMI, where both the SL stabilization mechanisms and magnetic ground states remain controversial. We address these here by investigating both the static and dynamical spin properties  ...

Energy-efficient, safe, and reliable Li-ion batteries (LIBs) are required for a wide range of applications. The introduction of ultra-thick graphite anodes, desired for high energy densities, meets limitations in internal electrode transport properties, leading to detrimental consequences. Yet, there is a lack of experimental tools capable of providing a complete view of local processes. Here, a multi-modal operando measurement approach is introduced, enabling quantitative spatio-temporal observations of Li concentrations and intercalation phases in ultra-thick graphite electrodes.
Neutron imaging and diffraction concurrently provide ...

The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe₂ is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetry Y and T points and disperse along the crystallographic b-axis. In applied magnetic fields ...

Methods to prepare and characterize neutron helical waves carrying orbital angular momentum (OAM) were recently demonstrated at small-angle neutron scattering (SANS) facilities. These methods enable access to the neutron orbital degree of freedom which provides new avenues of exploration in fundamental science experiments as well as in material characterization applications. 

However, ....

Additive manufacturing (AM) or “3D printing” of metals, which builds structure layer by layer, has revolutionized the production of intricate 3D designs. Among its techniques, laser powder bed fusion (PBF-LB) excels in creating metallic parts with intricate designs and high precision. This process can combine different metals into innovative multi-material components with tailored properties, with regards to e.g., strength and thermal conductivity, surpassing the capabilities of single-material designs. However, ....

Magnetic, thermodynamic, neutron diffraction and inelastic neutron scattering are used to study spin correlations in the easy-axis XXZ triangular lattice magnet K₂Co(SeO₃)₂. Despite the presence of quasi-2D “supersolid” magnetic order, the low-energy excitation spectrum contains no sharp modes and is instead a broad and structured multiparticle continuum. Applying a weak magnetic field ...

Topologically nontrivial magnetic structures such as skyrmion lattices are well known in materials lacking lattice inversion symmetry, where antisymmetric exchange interactions are allowed. Only recently, topological multi-q magnetic textures that spontaneously break the chiral symmetry, for example, three-dimensional hedgehog lattices, were discovered in centrosymmetric compounds, where they are instead driven by frustrated interactions. Here we show that ...

Quantum critical points (QCPs), zero-temperature phase transitions, are win- dows to fundamental quantum-mechanical phenomena associated with universal behaviour. Magnetic QCPs have been extensively investigated in the vicinity of antiferromagnetic order. However, QCPs are rare in metallic ferromagnets due to the coupling of the order parameter to electronic soft modes. Recently, antisymmetric spin-orbit coupling in noncentrosymmetric systems was suggested to protect ferromagnetic QCPs. Nonetheless, multiple centrosymmetric materials ...

The extraordinary properties of the Kitaev model have motivated an intense search for new physics in materials that combine geometrical and bond frustration. In this Letter, we employ inelastic neutron scattering, spin wave theory, and exact diagonalization to study the spin dynamics in the perfect triangular-lattice antiferromagnet (TLAF) CsCeSe₂. This material orders into a stripe phase, which is demonstrated to arise as a consequence of the off-diagonal bond-dependent terms in the spin Hamiltonian ...

The recent discovery of superconductivity in infinite layer thin films and bulk Ruddlesden–Popper nickelates has stimulated the investigation of other predicted properties of these materials. Among them, the existence of magnetism-driven ferroelectricity in the parent compounds RNiO₃ (R = 4f lanthanide and Y) at the onset of the Néel order, T_N, has remained particularly elusive. Using diffraction techniques, we reveal here the existence of magnetostriction at T_N in bulk YNiO₃ single crystals. Interestingly, the associated lattice anomalies ...

PSI Researcher used inelastic neutron scattering to show how collective lattice vibrations can be controlled by electric fields. These results indicate that different eigenmodes can couple in field in this incipient ferroelectric.

A hallmark of unconventional superconductors is a complex electronic phase diagram where intertwined orders of charge-spin-lattice degrees of freedom compete and coexist. While the kagome metals such as CsV₃Sb₅ also exhibit complex behavior, involving coexisting charge density wave order and superconductivity, much is unclear about the microscopic origin of the superconducting pairing. We study the vortex lattice in the superconducting state of Cs(V_0.86Ta_0.14)₃Sb₅, where the Ta-doping suppresses charge order and enhances superconductivity. Using small-angle neutron scattering ...

Van-der-Waals magnetic materials can be exfoliated to realize ultrathin sheets or interfaces with highly controllable optical or spintronics responses. In majority, these are collinear ferro-, ferri-, or antiferromagnets, with a particular scarcity of lattice-incommensurate helimagnets of defined left- or right-handed rotation sense, or helicity. Here, we report polarized neutron scattering experiments on DyTe₃, whose layered structure has highly metallic tellurium layers separated by double-slabs of dysprosium square nets...

Emergent quasiparticles with a Dirac dispersion in condensed matter systems can be described by the Dirac equation for relativistic electrons, in analogy with Dirac particles in high-energy physics. For example, electrons with a Dirac dispersion have been intensively studied in electronic systems such as graphene and topological insulators. However, charge is not a prerequisite for Dirac fermions, and the emergence of Dirac fermions without a charge degree of freedom has been theoretically predicted to be realized in Dirac quantum spin liquids. These quasiparticles ...

LiCu₃O₃ is an antiferromagnetic mixed valence cuprate where trilayers of edge-sharing Cu(II)O (3d⁹) are sandwiched in between planes of Cu(I) (3d¹⁰) ions, with Li stochastically substituting Cu(II). Angle-resolved photoemission spectroscopy (ARPES) and density functional theory reveal two insulating electronic subsystems that are segregated in spite of sharing common oxygen atoms: a Cu d_z²/O p_z derived valence band (VB) dispersing on the Cu(I) plane, and a Cu 3d_x²−y²/O 2p_x,y derived Zhang-Rice singlet (ZRS) band dispersing on the Cu(II)O planes.

We present high-quality angle-resolved photoemission (ARPES) and density functional theory calculations (DFT+U) of SmCoIn₅. We find broad agreement with previously published studies of LaCoIn₅ and CeCoIn₅, confirming that the Sm 4f electrons are mostly localized. Nevertheless, our model is consistent with an additional delocalized Sm component, stemming from hybridization between the 4f electrons and the metallic bands at “hot spot” positions in the Brillouin zone. 

The study presents a unique investigation of [Pt/CoFeB/Ru]₁₀ multilayers, revealing suppressed skyrmion phases, intricate magnetic domain structures, and Néel-type domain walls, providing crucial insights for spintronic applications.

In quantum magnetic materials, ordered phases induced by an applied mag- netic field can be described as the Bose-Einstein condensation (BEC) of mag- non excitations. In the strongly frustrated system SrCu₂(BO₃)₂, no clear magnon BEC could be observed, pointing to an alternative mechanism, but the high fields required to probe this physics have remained a barrier to detailed investigation.Here we exploit the first purpose-built high-field neutron scattering facility to measure ...