Here you find current and previous news from the PSI Center for Neutron and Muon Sciences.
In-situ visualization of stress-dependent bulk magnetic domain formation by neutron grating interferometry
The performance and degree of efficiency of industrial transformers are directly influenced by the magnetic properties of high-permeability steel laminations (HPSLs). Industrial transformer cores are built of stacks of single HPSLs. While the insulating coating on each HPSL reduces eddy-current losses in the transformer core, the coating also induces favorable inter-granular tensile stresses that significantly influence the underlying magnetic domain structure.
Rate of Molecular Transfer of Allyl Alcohol across an AOT Surfactant Layer Using Muon Spin Spectroscopy
The transfer rate of a probe molecule across the interfacial layer of a water-in-oil (w/o) microemulsion was investigated using a combination of transverse field muon spin rotation (TF-μSR), avoided level crossing muon spin resonance (ALC-μSR), and Monte Carlo simulations. Reverse micro-emulsions consist of nanometer-sized water droplets dispersed in an apolar solvent separated by a surfactant monolayer.
The flip-over effect in pulsed laser deposition: Is it relevant at high background gas pressures?
In pulsed laser deposition the use of a rectangular or elliptical beam spot with a non 1:1 aspect ratio leads to the so called flip-over effect. Here, the longest dimension of the laser spot results in the shortest direction of plasma plume expansion.
Nanostructure surveys of macroscopic specimens by small-angle scattering tensor tomography
The mechanical properties of many materials are based on the macroscopic arrangement and orientation of their nanostructure. This nanostructure can be ordered over a range of length scales. In biology, the principle of hierarchical ordering is often used to maximize functionality, such as strength and robustness of the material, while minimizing weight and energy cost.
Strong enhancement of s-wave superconductivity near a quantum critical point of Ca3Ir4Sn13
We report microscopic studies by muon spin rotation/relaxation as a function of pressure of the Ca3Ir4Sn13 and Sr3Ir4Sn13 cubic compounds, which are members of the (Ca1−xSrx)3Ir4Sn13 system displaying superconductivity and a structural phase transition associated with the formation of a charge density wave (CDW).
Direct evidence for a pressure-induced nodal superconducting gap in the Ba0.65Rb0.35Fe2As2 superconductor
The superconducting gap structure in iron-based high-temperature superconductors (Fe-HTSs) is non-universal. In contrast to other unconventional superconductors, in the Fe-HTSs both d-wave and extended s-wave pairing symmetries are close in energy. Probing the proximity between these very different superconducting states and identifying experi- mental parameters that can tune them is of central interest.
Intrinsic Paramagnetic Meissner Effect Due to s-Wave Odd-Frequency Superconductivity
In 1933, Meissner and Ochsenfeld reported the expulsion of magnetic flux - the diamagnetic Meissner effect - from the interior of superconducting lead. This discovery was crucial in formulating the Bardeen-Cooper-Schrieffer (BCS) theory of superconductivity. In exotic superconducting systems BCS theory does not strictly apply.
Visualizing the morphology of vortex lattice domains in a bulk type-II superconductor
Alike materials in the solid state, the phase diagram of type-II superconductors exhibit crystalline, amorphous, liquid and spatially inhomogeneous phases. The multitude of different phases of vortex matter has thence proven to act as almost ideal model system for the study of both the underlying properties of superconductivity but also of general phenomena such as domain nucleation and morphology.
Observation of Gravitationally Induced Vertical Striation of Polarized Ultracold Neutrons by Spin-Echo Spectroscopy
We describe a spin-echo method for ultracold neutrons (UCNs) confined in a precession chamber and exposed to a |B0| = 1μT magnetic field. We have demonstrated that the analysis of UCN spin-echo resonance signals in combination with knowledge of the ambient magnetic field provides an excellent method by which to reconstruct the energy spectrum of a confined ensemble of neutrons.
Response of Plasma-Polymerized Hexamethyldisiloxane Films to Aqueous Environments
Thin plasma polymer films were deposited in hexamethyldisiloxane (HMDSO) and HMDSO/O2 low-pressure discharges and their chemical structures analyzed using infrared (IR) spectroscopy and neutron reflectometry (NR). The (plasma-polymerized) ppHMDSO film exhibits hydrophobic, poly(dimethylsiloxane)-like properties, while the retention of carbon groups is reduced by O2 addition, yielding a more inorganic, hydrophilic ppSiOx film.
Remotely induced magnetism in a normal metal using a superconducting spin-valve
Superconducting spintronics has emerged in the past decade as a promising new field that seeks to open a new dimension for nanoelectronics by utilizing the internal spin structure of the superconducting Cooper pair as a new degree of freedom. Its basic building blocks are spin-triplet Cooper pairs with equally aligned spins, which are promoted by proximity of a conventional superconductor to a ferromagnetic material with inhomogeneous macroscopic magnetization.
Thermodynamic phase transitions in a frustrated magnetic metamaterial
Materials with interacting magnetic degrees of freedom display a rich variety of magnetic behaviour that can lead to novel collective equilibrium and out-of-equilibrium phenomena. In equilibrium, thermodynamic phases appear with the associated phase transitions providing a characteristic signature of the underlying collective behaviour.
Pressure-induced electronic phase separation of magnetism and superconductivity in CrAs
The recent discovery of pressure (p) induced superconductivity in the binary helimagnet CrAs has raised questions on how superconductivity emerges from the magnetic state and on the mechanism of the superconducting pairing. In the present work the suppression of magnetism and the occurrence of superconductivity in CrAs were studied by means of muon spin rotation.
Néel-type skyrmion lattice with confined orientation in the polar magnetic semiconductor GaV4S8
Following the early prediction of the skyrmion lattice (SkL) - a periodic array of spin vortices - it has been observed recently in various magnetic crystals mostly with chiral structure. Although non-chiral but polar crystals with Cnv symmetry were identified as ideal SkL hosts in pioneering theoretical studies, this archetype of SkL has remained experimentally unexplored.
Lattice dynamics of α-cristobalite and the Boson peak in silica glass
B. Wehinger et al., J. Phys.: Condens. Matter 27, 305401 (2015). This work marks a decisive step in the solution of the longstanding problem understanding the origin of the Boson peak in silica glass. The investigation by means of diffuse and inelastic x-ray scattering and lattice dynamics calculations from first principles allow for a direct comparison of the atomic motion in crystalline silica polymorphs and silica glass.
Candidate Quantum Spin Liquid in the Ce3+ Pyrochlore Stannate Ce2Sn2O7
We report the low-temperature magnetic properties of Ce2Sn2O7, a rare-earth pyrochlore. Our suscep- tibility and magnetization measurements show that due to the thermal isolation of a Kramers doublet ground state, Ce2Sn2O7 has Ising-like magnetic moments of ∼1.18 μB. The magnetic moments are confined to the local trigonal axes, as in a spin ice, but the exchange interactions are antiferromagnetic.
Beating the Stoner criterion using molecular interfaces
Only three elements are ferromagnetic at room temperature: the transition metals iron, cobalt and nickel. The Stoner criterion explains why iron is ferromagnetic but manganese, for example, is not, even though both elements have an unfilled 3d shell and are adjacent in the periodic table: according to this criterion, the product of the density of states and the exchange integral must be greater than unity for spontaneous spin ordering to emerge.
Evidence for Coexistence of Bulk Superconductivity and Itinerant Antiferromagnetism in the Heavy Fermion System CeCo(In1−xCdx)5
In the generic phase diagram of heavy fermion systems, tuning an external parameter such as hydrostatic or chemical pressure modifies the superconducting transition temperature. The superconducting phase forms a dome in the temperature-tuning parameter phase diagram, which is associated with a maximum of the superconducting pairing interaction. Proximity to antiferromagnetism suggests a relation between the disappearance of antiferromagnetic order and superconductivity.
A new class of chiral materials hosting magnetic skyrmions beyond room temperature
Skyrmions, topologically protected vortex-like nanometric spin textures in magnets, have been attracting increasing attention for emergent electromagnetic responses and possible technological applications for spintronics. In particular, metallic magnets with chiral and cubic/tetragonal crystal structure may have high potential to host skyrmions that can be driven by low electrical current excitation.
Interplay between magnetic order at Mn and Tm sites alongside the structural distortion in multiferroic films of o-TmMnO3
We employ resonant soft x-ray diffraction to individually study the magnetic ordering of the Mn and the Tm sublattices in single-crystalline films of orthorhombic (o−)TmMnO3. The same magnetic ordering wave vector of (0q0) with q≈0.46 is found for both ionic species, suggesting that the familiar antiferromagnetic order of the Mn ions induces a magnetic order on the Tm unpaired 4f electrons.
Crystallization of zirconia based thin films
In pulsed laser deposition the use of a rectangular or elliptical beam spot with a non 1:1 aspect ratio leads to the so called flip-over effect. Here, the longest dimension of the laser spot results in the shortest direction of plasma plume expansion.
Mutual Independence of Critical Temperature and Superfluid Density under Pressure in Optimally Electron-Doped Superconducting LaFeAsO1−xFx
The superconducting properties of LaFeAsO1−xFx under conditions of optimal electron doping are investigated upon the application of external pressure up to ∼23 kbar. Measurements of muon-spin spectroscopy and dc magnetometry evidence a clear mutual independence between the critical temperature Tc and the low-temperature saturation value for the ratio ns/m* (superfluid density over effective band mass of Cooper pairs).
Spin-stripe phase in a frustrated zigzag spin-1/2 chain
Motifs of periodic modulations are encountered in a variety of natural systems, where at least two rival states are present. In strongly correlated electron systems, such behaviour has typically been associated with competition between short- and long-range interactions, for example, between exchange and dipole-dipole interactions in the case of ferromagnetic thin films.
Magnetoelectric domain control in multiferroic TbMnO3
The manipulation of domains by external fields in ferroic materials is of major interest for applications. In multiferroics with strongly coupled magnetic and electric order, however, the magnetoelectric coupling on the level of the domains is largely unexplored. We investigated the field-induced domain dynamics of TbMnO3 in the multiferroic ground state and across a first-order spin-flop transition.
Constraining interactions mediated by axion-like particles with ultracold neutrons
We report a new limit on a possible short range spin-dependent interaction from the precise measurement of the ratio of Larmor precession frequencies of stored ultracold neutrons and 199Hg atoms confined in the same volume. The measurement was performed in a ∼1μT vertical magnetic holding field with the apparatus searching for a permanent electric dipole moment of the neutron at the Paul Scherrer Institute.
Controllable Broadband Absorption in the Mixed Phase of Metamagnets
Materials with broad absorption bands are highly desirable for electromagnetic filtering and processing applications, especially if the absorption can be externally controlled. Here, a new class of broadband-absorption materials is introduced. Namely, layered metamagnets exhibit an electromagnetic excitation continuum in the magnetic-field-induced mixed ferro- and antiferromagnetic phase.
Observation of the rare BS0 →μ+μ- decay from the combined analysis of CMS and LHCb data
The standard model of particle physics describes the fundamental particles and their interactions via the strong, electromagnetic and weak forces. It provides precise predictions for measurable quantities that can be tested experimentally. The probabilities, or branching fractions, of the strange B meson (BS0) and the B0 meson decaying into two oppositely charged muons (μ+ and μ-) are especially inter- esting because of their sensitivity to theories that extend the standard model. The standard model predicts that the BS0 →μ+μ- and B0 →μ+μ- decays are very rare, with about four of the former occurring for every billion Bs0 mesons produced, and one of the latter occurring for every ten billion B0 mesons.
Isotopically-enriched gadolinium-157 oxysulfide scintillator screens for the high-resolution neutron imaging
High-resolution neutron imaging (Neutron Microscope project) requires highly efficient scintillator screens. Our aim is to achieve sub-5µm spatial resolution. Here, we demonstrate the feasibility of the production of isotopically-enriched gadolinium oxysulfide scintillator screens for the high spatial-resolution neutron imaging. Approximately 10 g of 157Gd2O2S:Tb was produced in the form of fine powder (the level of 157Gd enrichment above 88%).
Structural and Magnetic Phase Transitions near Optimal Superconductivity in BaFe2(As1-xPx)2
We use nuclear magnetic resonance (NMR), high-resolution x-ray, and neutron scattering studies to study structural and magnetic phase transitions in phosphorus-doped BaFe2(As1-xPx)2. Previous transport, NMR, specific heat, and magnetic penetration depth measurements have provided compelling evidence for the presence of a quantum critical point (QCP) near optimal superconductivity at x=0.3.
Mass Density and Water Content of Saturated Never-Dried Calcium Silicate Hydrates
Calcium silicate hydrates (C-S-H) are the most abundant hydration products in ordinary Portland cement paste. Yet, despite the critical role they play in determining mechanical and transport properties, there is still a debate about their density and exact composition. Here, the site-specific mass density and composition of C-S-H in hydrated cement paste are determined with nanoscale resolution in a nondestructive approach.