CNM - Publication Highlights

The interplay between oxygen and spin ordering for the low oxygen doped Nd₂NiO_4.10 has been investigated by single-crystal neutron diffraction. We find a coexistence of the magnetic order below T_N  with the 3D ordering of excess oxygen atoms, which has not been previously observed for the homologous nickelates. Moreover, the magnetic ordering modulation vectors are no longer independent and exactly follow the modulation vectors of the oxygen ordering.

A better understanding of quantum spin liquids (QSLs), where spin dimer configurations are fluctuating even at the low- est temperatures, could be of use in quantum information, in superconducting or other technologies. This macroscopic collective state typically arises from geometrical frustration or low dimensionality. In the layered EDT-BCO, we report a QSL state, which is generated, on different bases, with the intrinsic disorder.

Quantum spin liquids are materials that feature quantum entangled spin correlations and avoid magnetic long-range order at T =0 K. Particularly interesting are two-dimensional honeycomb spin lattices where a plethora of exotic quantum spin liquids have been predicted. Here, we experimentally study an effective S = 1/2 Heisenberg honeycomb lattice with competing nearest and next-nearest-neighbour interactions.

Magnetic skyrmions are well-suited for encoding information because they are nano-sized, topologically stable, and only require ultra-low critical current densities j_c to depin from the underlying atomic lattice. Above j_c, skyrmions exhibit well-controlled motion, making them prime candidates for race-track memories. In thin films thermally-activated creep motion of isolated skyrmions was observed below j_c as predicted by theory.

Magnetic skyrmion is a topologically protected particle-like object in magnetic materials, appearing as a nanometric swirling spin texture. The size and shape of skyrmion particles can be flexibly controlled by external stimuli, which suggests unique features of their crystallization and lattice transformation process. Here, we investigated the detailed mechanism of structural transition of skyrmion lattice (SkL) in a prototype chiral cubic magnet Cu₂OSeO₃, by combining resonant soft X-ray scattering (RSXS) experiment and micromagnetic simulation...

Quantum materials have properties that defy conventional theories of solids. Explaining these unusual properties is a frontier in physics, which promises both technological applications and fundamentally new states of matter. Yb₂Ti₂O₇ is a center of attention in this work. While it becomes ferromagnetic at very low temperature, its excitation spectrum resembles that of a quantum spin liquid. We show using neutron scattering ...

Non-centrosymmetric superconductors (NCSCs) are promising candidates in the search for unconventional and topological superconductivity. The α-Mn-type rhenium-based alloys represent excellent examples of NCSCs, where spontaneous magneticfields, peculiar to time-reversal symmetry (TRS) breaking, have been shown to develop in the superconducting phase. By converse, TRS is preserved in many other isostructural NCSCs, thus leaving the key question about its origin fully open. Here, we consider ...

We report a comprehensive muon spectroscopy study of the Zn-barlowite series of S=1/2 kagomé antiferromagnets, Zn_xCu_4−x(OH)₆FBr, for x = 0.00 to 0.99(1). By combining muon spin relaxation and rotation measurements with state-of-the-art density-functional theory muon-site calculations, we observe the formation of both μ–F and μ–OH complexes in Zn-barlowite. From these stopping sites, implanted muon spins reveal the suppression of long-range magnetic order into a possible quantum spin liquid state upon the increasing concentration of Zn-substitution.

In the past years, the strategies used to break the Cu(In,Ga)Se₂ (CIGS) light to power conversion effi- ciency world record value were based on improvements of the absorber optoelectronic and crystalline properties, mainly using complex post-deposition treatments. To reach even higher efficiency values, fur- ther advances in the solar cell architecture are needed, in particular, with respect to the CIGS interfaces. In this study, we evaluate the structural, morphological and optoelectronic impact of an Al₂O₃ layer as a potential front passivation layer on the CIGS properties, as well as an Al₂O₃ tunneling layer between CIGS and CdS.

We demonstrate efficient transverse compression of a 12.5 MeV=c muon beam stopped in a helium gas target featuring a vertical density gradient and crossed electric and magnetic fields. The muon stop distribution extending vertically over 14 mm was reduced to a 0.25 mm size (rms) within 3.5 μs. The simulation including cross sections ...

3D magnetic nanostructures are of great interest due to the possibility to design novel properties and the benefits for both technological applications such as high-density data storage, as well as more fundamental studies.

One of the main challenges facing the realization of these three-dimensional systems is their fabrication, which includes the deposition of magnetic materials on 3D surfaces. In this work, the electroless deposition of Ni–Fe

on a 3D-printed, non-conductive microstructure is presented.

In the three-dimensional (3D) Heisenberg model, topological point defects known as spin hedgehogs behave as emergent magnetic monopoles, i.e., quantized sources and sinks of gauge fields that couple strongly to conduction electrons, and cause unconventional transport responses such as the gigantic Hall effect. We observe a dramatic change in the Hall effect upon the transformation of a spin hedgehog crystal in a chiral magnet MnGe through combined measurements of magnetotransport and small-angle neutron scattering (SANS).

Magnetic skyrmions are topological solitons with a nanoscale winding spin texture that hold promise for spintronics applications. Skyrmions have so far been observed in a variety of magnets that exhibit nearly parallel alignment for neighbouring spins, but theoretically skyrmions with anti-parallel neighbouring spins are also possible. Such antiferromagnetic skyrmions may allow more flexible control than conventional ferromagnetic skyrmions. Here, by combining neutron scattering measurements and Monte Carlo simulations, we show that a fractional antiferromagnetic skyrmion lattice is stabilized in MnSc₂S₄ through anisotropic couplings.

Understanding the relationship between entangled degrees of freedom (DOF) is a central problem in correlated materials and the possibility to influence their balance is promising toward realizing novel functionalities. In Sr₂IrO₄, the interaction between spin–orbit coupling and electron correlations induces an exotic ground state with magnetotransport properties promising for antiferromagnetic spintronics applications.

Quantum states induced by single-atomic impurities are at the frontier of physics and material science. While such states have been reported in high-temperature superconductors and dilute magnetic semiconductors, they are unexplored in topological magnets which can feature spin-orbit tunability. Here we use spin-polarized scanning tunneling microscopy/ spectroscopy (STM/S) to study the engineered quantum impurity in a topological magnet Co3Sn2S2. We find that each substituted In impurity introduces a striking localized bound state.

Recently, discrepancies of up to 4σ between the different determinations of the Cabibbo angle were observed. In this context, we point out that this “Cabibbo-angle anomaly” can be explained by lepton flavor universality violating new physics in the neutrino sector. However, modified neutrino couplings to standard model gauge bosons also affect many other observables sensitive to lepton flavor universality violation, which have to be taken into account in order to assess the viability of this explanation.

The driving force in materials to spontaneously form states with magnetic or electric order is of fundamental importance for basic research and device technology. The macroscopic properties and functionalities of these ferroics depend on the size, distribution and morphology of domains; that is, of regions across which such uniform order is maintained. Typically, extrinsic factors such as strain profiles, grain size or annealing procedures control the size and shape of the domains, whereas intrinsic parameters are often difficult to extract due to the complexity of a processed material. Here, we achieve this separation ...

Here we investigate antiferromagnetic Eu₅In₂Sb₆, a nonsymmorphic Zintl phase. Our electrical transport data show that Eu₅In₂Sb₆ is remarkably insulating and exhibits an exceptionally large negative magnetoresistance, which is consistent with the presence of magnetic polarons. From ab initio calculations, the paramagnetic state of Eu₅In₂Sb₆ is a topologically nontrivial semimetal within the generalized gradient approximation (GGA), whereas an insulating state with trivial topological indices is obtained using a modified Becke−Johnson potential.

We use scanning tunneling microscopy to elucidate the atomically resolved electronic structure in the strongly correlated kagome Weyl antiferromagnet Mn₃Sn. In stark contrast to its broad single-particle electronic structure, we observe a pronounced resonance with a Fano line shape at the Fermi level resembling the many-body Kondo resonance. We find that this resonance does not arise from the step edges or atomic impurities but the intrinsic kagome lattice.

It has recently been proposed that combining chirality with topological band theory results in a totally new class of fermions. Understanding how these unconventional quasiparticles propagate and interact remains largely unexplored so far. Here, we use scanning tunneling microscopy to visualize the electronic properties of the prototypical chiral topological semimetal PdGa.

Noncollinear magnetic order arises for various reasons in several magnetic systems and exhibits interesting spin dynamics. Despite its ubiquitous presence, little is known of how magnons, otherwise stable quasiparticles, decay in these systems, particularly in metallic magnets. Using inelastic neutron scattering, we examine the magnetic excitation spectra in a metallic noncollinear antiferromagnet CrB₂, in which Cr atoms form a triangular lattice and display incommensurate magnetic order. Our data show intrinsic magnon damping ...