Energie et climat

Here we use in-situ high-temperature x-ray absorption spectroscopy (XAS) and theoretical calculations to quantify the amorphous structure of bulk and nanoscale GeTe. Based on XAS experiments, we develop a theoretical model of the amorphous GeTe structure, consisting of a disordered fcc-type Te sublattice and randomly arranged chains of Ge atoms in a tetrahedral coordination.

Infrared spectroscopy (IR) is a widely used technique enabling to identify specific functional groups in the molecule of interest based on their characteristic vibrational modes or the presence of a specific adsorption site based on the characteristic vibrational mode of an adsorbed probe molecule. The interpretation of an IR spectrum is generally carried out within a fingerprint paradigm by comparing the observed spectral features with the features of known references or theoretical calculations. This work demonstrates a method for extracting quantitative structural information beyond this approach by application of machine learning (ML) algorithms.

A study involving PSI scientists from the LMS lab, and just published in Physical Review Letters has found that in manganese oxide, a textbook antiferromagnetic material,  the site of an implanted spin-polarized muon is not well identified, but can change due to a previously neglected effect: magnetostriction.

Magnetostriction results from the coupling between magnetic and elastic degrees of freedom. Though it is associated with a relatively small energy, we show that it plays an important role in determining the site of an implanted muon, so that the energetically favorable site can switch on crossing a magnetic phase transition. This surprising effect is demonstrated in the cubic rocksalt antiferromagnet MnO which undergoes a magnetostriction-driven rhombohedral distortion at the Néel temperature T_N = 118 K. Above T_N ...

On January 23rd, 2024, first "Swedish" X-ray light was delivered to the SOPHIE endstation, currently installed at the SoftiMAX beamline of the MaxIV light source.

n2EDM is the current state of the art experiment carrying out a high-precision search for an electric dipole moment of the neutron at the ultra-cold neutron source of PSI. In order to reach it’s incredible precision of 10^-27 e cm, a stable and uniform magnetic environment is critical. Thus, shielding the experiment from external magnetic flux and preparing a pristine magnetic environment is crucial. To achieve this, n2EDM uses both passive and active magnetic shielding components. External, or residual, magnetic field contributions must be near-zero, and can be achieved via “degaussing” the experiment’s passive magnetic shielding. Degaussing reduces, ideally “erases”, the residual magnetization of a material. In this work, we greatly improved the degaussing procedure of n2EDM, reducing the residual magnetic field by a factor of two, improving its uniformity, and all while taking less time and dissipating less heat.

Synchrotron X-ray diffraction sheds  light on laser-induced local recrystallization .

In quantum magnetic materials, ordered phases induced by an applied mag- netic field can be described as the Bose-Einstein condensation (BEC) of mag- non excitations. In the strongly frustrated system SrCu₂(BO₃)₂, no clear magnon BEC could be observed, pointing to an alternative mechanism, but the high fields required to probe this physics have remained a barrier to detailed investigation.Here we exploit the first purpose-built high-field neutron scattering facility to measure ...

Pt-FeO_x(OH)_y interface with enhanced activity for PROX is generated via strong metal-support interaction. Increase in the degree of hydroxylation of Pt-FeO_x(OH)_y interface enhances the rate of PROX mediated by active Fe²⁺ species.

Understanding the degree to which charge-stripe, spin-stripe, and superconducting orders compete/coexist is paramount for elucidating the microscopic pairing mechanism in the cuprate high-temperature superconductors. We explore the tunability of magnetism, superconductivity, and crystal structure in the stripe phase of the cuprate La_2−xBa_xCuO₄, by employing complementary techniques under compressive uniaxial stress in the CuO₂ plane. Our results show a sixfold increase ...