Energy transition

Shifting away from nuclear energy, expanding solar and wind power, generating energy from biomass, reducing energy consumption. Switzerland is committed to becoming climate-neutral by 2050. An ambitious goal, which has become more urgent than ever due to the increasingly challenging geopolitical situation. How can a sustainable and resilient energy supply for Switzerland be established over the coming years? What's the optimal way to use renewable energy sources? What new technologies are especially promising? At PSI, researchers are seeking answers to these crucial questions.

Terahertz spot size before (left) and after (right) wavefront optimization

Terahertz wavefront control for extremely bright THz bullet

The brightness of a light source defines its applicability to nonlinear phenomena in science. The SwissFEL laser group has now overcome one of the two principal technological hurdles to produce bright pulses in the Terahertz range (0.1-5 THz).

Competing superconducting and magnetic order parameters and field-induced magnetism in electron-doped Ba(Fe1-xCox)2As2

We have studied the magnetic and superconducting properties of Ba(Fe0.95Co0.05)2As2 as a function of temperature and external magnetic field using neutron scattering and muon spin rotation. Below the superconducting transition temperature the magnetic and superconducting order parameters coexist and compete. A magnetic field can significantly enhance the magnetic scattering in the superconducting state, roughly doubling the Bragg intensity at 13.5T.

Magnetization dynamics inside a 5 µm x 5 µm structure.(a) Time-resolved PEEM images using XMCD as a magnetic contrast mechanism recorded at a given time delay t after the laser pulse and (b) extracted XMCD contrast as a function of the time delay t for three different ROI, defined in the inset image by the coloured area superimposed on the non-dichroic X-ray absorption of the structure. The 0° incoming laser direction with respect to the structure edge is indicated in the inset by the laser in-plane wave v…

Nanoscale sub-100 picosecond all-optical magnetization switching in GdFeCo microstructure

Ultrafast magnetization reversal driven by femtosecond laser pulses has been shown to be a promising way to write information. Seeking to improve the recording density has raised intriguing fundamental questions about the feasibility of combining ultrafast temporal resolution with sub-wavelength spatial resolution for magnetic recording. Here we report on the experimental demonstration of nanoscale sub-100 ps all-optical magnetization switching, providing a path to sub-wavelength magnetic recording.

Magnetic moment measured by XMCD and resistivity as a funtion of temperature for two different piezostrain states

Control of Tc in La0.7Sr0.3MnO3 via piezostrain

X-ray magnetic circular dichroism measurements evidence a 10K shift of the magnetic Curie temperature for La0.7Sr0.3MnO3 deposited on the piezoelectric substrate [Pb(Mg1/3Nb2/3)O3]0.68−[PbTiO3]0.32 (011) for two different remanent piezostrain states.

Anisotropic Local Modification of Crystal Field Levels in Pr-Based Pyrochlores: A Muon-Induced Effect Modeled Using Density Functional Theory

Although muon spin relaxation is commonly used to probe local magnetic order, spin freezing, and spin dynamics, we identify an experimental situation in which the measured response is dominated by an effect resulting from the muon-induced local distortion rather than the intrinsic behavior of the host compound.

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PSI summer school 2015

The PSI summer school 2015 on Condensed Matter Research will be organized at the Lyceum Alpinum in Zuoz, Switzerland from August 15-21, 2015. International experts and PSI staff members will introduce and deepen your knowledge not only on methods but also on those phenomena, which are presently at the forefront of modern solid state physics and chemistry. The school will be followed by hands-on practical training at the PSI large user facilities SINQ, SμS and SLS. Online registration and detailed information is available from the school's webpage.

Coexistence of 3d-Ferromagnetism and Superconductivity in [(Li1-Fex)OH](Fe1-yLiy)Se

Superconducting [(Li1-xFex)OH](Fe1-yLiy)Se (x≈0.2, y≈0.08) was synthesized by hydrothermal methods and characterized by single-crystal and powder X-ray diffrac- tion. The structure contains alternating layers of anti-PbO type (Fe1-yLiy)Se and (Li1-xFex)OH. Electrical resistivity and magnetic susceptibility measurements reveal superconductivity at 43K.

Fractional excitations in the square-lattice quantum antiferromagnet

Quantum magnets have occupied the fertile ground between many-body theory and low-temperature experiments on real materials since the early days of quantum mechanics. However, our understanding of even deceptively simple systems of interacting spin-1/2 particles is far from complete. The quantum square-lattice Heisenberg antiferromagnet, for example, exhibits a striking anomaly of hitherto unknown origin in its magnetic excitation spectrum.

A measurement of the neutron to 199Hg magnetic moment ratio

The neutron gyromagnetic ratio has been measured relative to that of the 199Hg atom with an uncertainty of 0.8 ppm. We employed an apparatus where ultracold neutrons and mercury atoms are stored in the same volume and report the result γnHg = 3.8424574(30).

Short-Range Correlations in the Magnetic Ground State of Na4Ir3O8

The magnetic ground state of the Jeff = 1/2 hyperkagome lattice in Na4Ir3O8 is explored via combined bulk magnetization, muon spin relaxation, and neutron scattering measurements. A short-range, frozen state comprised of quasistatic moments develops below a characteristic temperature of TF = 6K, revealing an inhomogeneous distribution of spins occupying the entirety of the sample volume. Quasistatic, short- range spin correlations persist until at least 20 mK and differ substantially from the nominally dynamic response of a quantum spin liquid. Our data demonstrate that an inhomogeneous magnetic ground state arises in Na4Ir3O8 driven either by disorder inherent to the creation of the hyperkagome lattice itself or stabilized via quantum fluctuations.

Measurement of the parameter ξ″ in polarized muon decay and implications on exotic couplings of the leptonic weak interaction

The muon decay parameter ξ″ has been determined in a measurement of the longitudinal polarization of positrons emitted from polarized and depolarized muons. The result, ξ″ = 0.981 ± 0.045stat ± 0.003syst, is consistent with the Standard Model prediction of unity, and provides an order of magnitude improvement in the relative precision of this parameter. This value sets new constraints on exotic couplings beyond the dominant V-A description of the leptonic weak interaction.

Innovation Award on Synchrotron Radiation 2014 for high-resolution 3D hard X-ray microscopy

The 2014 Innovation Award on Synchrotron Radiation was bestowed to researchers Ana Diaz, Manuel Guizar-Sicairos, Mirko Holler, and Jörg Raabe from the Paul Scherrer Institut, Switzerland, for their contributions to method and instrumentation development, which have set new standards in high-resolution 3D hard X-ray microscopy.

k=0 Magnetic Structure and Absence of Ferroelectricity in SmFeO3

SmFeO3 has attracted considerable attention very recently due to its reported multiferroic properties above room temperature. We have performed powder and single crystal neutron diffraction as well as complementary polarization dependent soft X-ray absorption spectroscopy measurements on floating-zone grown SmFeO3 single crystals in order to determine its magnetic structure. We found a k=0 G-type collinear antiferromagnetic structure that is not compatible with inverse Dzyaloshinskii-Moriya interaction driven ferroelectricity. While the structural data reveal a clear sign for magneto-elastic coupling at the Néel-temperature of ∼675 K, the dielectric measurements remain silent as far as ferroelectricity is concerned.

A high-pressure hydrogen time projection chamber for the MuCap experiment

The MuCap experiment at the Paul Scherrer Institute performed a high-precision measurement of the rate of the basic electroweak process of nuclear muon capture by the proton, μ- + p → n + νμ. The experimental approach was based on the use of a time projection chamber (TPC) that operated in pure hydrogen gas at a pressure of 10 bar and functioned as an active muon stopping target. The TPC detected the tracks of individual muon arrivals in three dimensions, while the trajectories of outgoing decay (Michel) electrons were measured by two surrounding wire chambers and a plastic scintillation hodoscope.

Molecular Scale Dynamics of Large Ring Polymers

We present neutron scattering data on the structure and dynamics of melts from polyethylene oxide rings with molecular weights up to ten times the entanglement mass of the linear counterpart. The data reveal a very compact conformation displaying a structure approaching a mass fractal, as hypothesized by recent simulation work. The dynamics is characterized by a fast Rouse relaxation of subunits (loops) and a slower dynamics displaying a lattice animal-like loop displacement.

Temperature dependence of the (050) reflection from a 200 nm o−LuMnO3 [110]-oriented film. Inset (a): Temperature dependence of the integrated intensity from the (050) structural reflection (black) and the (0qb≈½0) magnetic reflection (red) of this film. Inset (b): The simplest approximation for a distortion producing nonzero intensity for a (0k0) reflection with k odd, depicted for two atoms along the b direction.

Multiferroic Properties of o−LuMnO3 Controlled by b-Axis Strain

Strain is a leading candidate for controlling magnetoelectric coupling in multiferroics. Here, we use x-ray diffraction to study the coupling between magnetic order and structural distortion in epitaxial films of the orthorhombic (o-) perovskite LuMnO3. An antiferromagnetic spin canting in the E-type magnetic structure is shown to be related to the ferroelectrically induced structural distortion and to a change in the magnetic propagation vector.

Structural and magnetic dynamics in the magnetic shape-memory alloy Ni2MnGa

Magnetic shape-memory Heusler alloys are multiferroics stabilized by the correlations between electronic, magnetic, and structural order. To study these correlations we use time-resolved x-ray diffraction and magneto-optical Kerr effect experiments to measure the laser induced dynamics in a Heusler alloy Ni2MnGa film and reveal a set of time scales intrinsic to the system.