Energiewende

Abkehr von der Kernenergie, Ausbau von Solar- und Windkraft, Energiegewinnung aus Biomasse, Senkung des Energieverbrauchs. Bis 2050 soll die Schweiz klimaneutral werden. Ein ehrgeiziges Ziel, welches durch die zunehmend herausfordernde geopolitische Lage dringlicher denn je geworden ist. Wie lässt sich in den nächsten Jahren eine nachhaltige und widerstandsfähige Energieversorgung für die Schweiz aufbauen? Wie können erneuerbare Energien optimal genutzt werden? Welche neuen Technologien sind besonders vielversprechend? Am PSI suchen Forschende nach Antworten auf diese entscheidenden Fragen.

Laser spectroscopy of muonic deuterium

The deuteron is the simplest compound nucleus, composed of one proton and one neutron. Deuteron properties such as the root-mean-square charge radius rd and the polarizability serve as important benchmarks for understanding the nuclear forces and structure. Muonic deuterium μd is the exotic atom formed by a deuteron and a negative muon μ-.

Mini control room SwissFEL building

First Free Electrons at SwissFEL

At SwissFEL the first free electrons were produced and accelerated to 7.9 MeV. The electrons were stopped directly after the gun in the gun-spectrometer. The bunch charge was 20-50pC, with a repition rate of 10Hz. First measurements showed that the generated electron beam was of high quality. This means that the first milestone for the SwissFEL beam commissioning was reached!

Search for the lepton flavour violating decay μ+→e+γ with the full dataset of the MEG experiment

The final results of the search for the lepton flavour violating decay μ+→e+γ based on the full dataset collected by the MEG experiment at the Paul Scherrer Institut in the period 2009–2013 and totalling 7.5×1014 stopped muons on target are presented.

Sketch of a ferroic triangle showing the relation and techniques with which the ferroic orders, FM, AFM, and FE, and their mutual coupling have been established. The experimental techniques written in black letters (polarized neutron reflectometry, PNR; resonant soft x-ray diffraction, SXRD; x-ray diffraction, XRD) to identify ferroic properties have been reported elsewhere [22, 24]. Magnetization, susceptibility, μSR, neutron diffraction, and electrical polarization are reported.

Coexisting multiple order parameters in single-layer LuMnO3 films

Magnetoelectric multiferroics hold great promise for electrical control of magnetism or magnetic control of ferroelectricity. However, single phase ferroelectric materials with a sizeable ferromagnetic magnetization are rare. Here, we demonstrate that a single-phase orthorhombic LuMnO3 thin film features coexisting magnetic and ferroelectric orders.

The injector shoots tiny protein crystals into the beam of X-ray pulses. Per experiment, it requires only a few milligrams of the precious crystals. (Photo: Paul Scherrer Institute/Mahir Dzambegovic)

Catching proteins in the act

Some of the fastest processes in our body run their course in proteins activated by light. The protein rhodopsin sees to it that our eyes can rapidly take in their ever-changing surroundings. Free-electron X-ray lasers such as SwissFEL at the Paul Scherrer Institute PSI now make it possible for the first time to catch such processes in flagranti. Free-electron X-ray lasers generate extremely short and intense pulses of X-ray light.

(a) The dichroic ptychography setup. A diamond phase plate converts linearly polarized light into CL or CR light, which is then focused close to the sample plane. A piezoelectric stage is used to scan the sample across the beam. (b) The absorption part of reconstructed images taken with CL and CR polarized light at the Gd L3 edge with a photon energy of 7.2445 keV, which contain both electron density and magnetic contributions. The difference of these images removes the electron density contrast of Pt refe…

High-resolution hard x-ray magnetic imaging with dichroic ptychography

Imaging the magnetic structure of a material is essential to understanding the influence of the physical and chemical microstructure on its magnetic properties. Magnetic imaging techniques, however, have been unable to probe three-dimensional micrometer-size systems with nanoscale resolution. Here we present the imaging of the magnetic domain configuration of a micrometer-thick FeGd multilayer with hard x-ray dichroic ptychography at energies spanning both the Gd L3 edge and the Fe K edge, providing a high spatial resolution spectroscopic analysis of the complex x-ray magnetic circular dichroism.

Volume-wise destruction of the antiferromagnetic Mott insulating state through quantum tuning

RENiO3 (RE=rare-earth element) and V2O3 are archetypal Mott insulator systems. When tuned by chemical substitution (RENiO3) or pressure (V2O3), they exhibit a quantum phase transition (QPT) between an antiferromagnetic Mott insulating state and a paramagnetic metallic state. Because novel physics often appears near a Mott QPT, the details of this transition, such as whether it is first or second order, are important.

T2R-TTL.jpg

Call for expressions of interest: Beamline partners at the SLS for PX II and PX III

We invite companies and institutions to secure access to the beamlines X10SA/PX II and X06DA/PX III through a long term contract.

On the Interaction between Digitonin and Cholesterol in Langmuir Monolayers

In this article, we describe the effect of a highly hemolytic saponin, digitonin, on model lipids cholesterol and dipalmitoylphosphatidylcholine (DPPC) using a combination of tensiometric (surface pressure and dilatational surface elasticity), spectroscopic (infrared reflection absorption spectroscopy, IRRAS), microscopic (fluorescence microscopy), and scattering techniques (neutron reflectivity, NR, and grazing incidence X-ray diffraction, GIXD).

Mougel 2016 CS.jpg

Low temperature activation of supported metathesis catalysts by organosilicon reducing agents

Industrial alkene metathesis processes rely on silica-supported tungsten oxide catalysts, which operate at high temperatures (>350 °C) due to the difficulty in generating active sites (carbenes or metallacyclobutanes). We report here a low temperature activation process of well-defined metal oxo surface species using organosilicon reductants, which generate a large amount of active species at only 70 °C (0.6 active sites/W).

Phononic Structure Engineering: the Realization of Einstein Rattling in Calcium Cobaltate for the Suppression of Thermal Conductivity

Phonons in condensed matter materials transmit energy through atomic lattices as coherent vibrational waves. Like electronic and photonic properties, an improved understanding of phononic properties is essential for the development of functional materials, including thermoelectric materials. Recently, an Einstein rattling mode was found in thermoelectric material Na0.8CoO2, due to the large displacement of Na between the [CoO2] layers.

Physical realization of a quantum spin liquid based on a complex frustration mechanism

Unlike conventional magnets where the magnetic moments are partially or completely static in the ground state, in a quantum spin liquid they remain in collective motion down to the lowest temperatures. The importance of this state is that it is coherent and highly entangled without breaking local symmetries.

Iridates from the molecular side

New exotic phenomena have recently been discovered in oxides of paramagnetic Ir4+ ions, widely known as ‘iridates’. Their remarkable properties originate from concerted effects of the crystal field, magnetic interactions and strong spin-orbit coupling, characteristic of 5d metal ions.

Magnetic hysteresis of a submonolayer of TbPc2 molecules on magnesium oxide.

Magnesium Oxide Boosts the Hysteresis of Single-Molecule Magnets

Researchers from PSI and EPFL have demonstrated that the magnetization hysteresis and remanence of TbPc2 single-molecule magnets drastically depends on the substrate on which they are deposited. If a few atomic layers thick magnesium oxide film grown on a silver substrate is used, a record wide hysteresis and record large remanence can be obtained. Single-molecule magnets are attractive for molecular spintronics applications such as information processing or storage.

Spin-wave.jpg

A Mini-Antenna for the Data Processing of Tomorrow

The use of spin-wave signals in future information processing devices can substantially reduce power consumption over present charge current based technologies. As part of an international research venture, scientists at PSI now introduced a concept to generate spin waves with nanoscale wavelengths exploiting the driven dynamics of magnetic vortex cores in magnetic heterostructures.

POLAR detector developed at the PSI flies into orbit with a Chinese space mission

Researchers working with Wojciech Hajdas at the Paul Scherrer Institute PSI have developed a detector called POLAR. This instrument is expected to search out and investigate so-called gamma ray bursts coming from the depths of the universe. Gamma ray bursts are eruptions of high-energy light that despite being extremely strong remain, up to now, only poorly understood.

Shedding light on the origins of high-Tc superconductivity in bismuth oxides

Researchers have overcome a number of challenges in order to employ an advanced probe in the study of an unusual material, barium bismuth oxide (BaBiO3) – an insulating parent compound of a family of high-temperature superconductors known since the late 80s. In order to finally realize the experiments, the researchers grew and studied thin films of the material completely in situ under ultrahigh vacuum conditions. The results show that superconductivity in bismuth oxides emerges out of a novel insulating phase, where hole pairs located on combinations of the oxygen orbitals are coupled with distortions of the crystal lattice.

Muon polarization in the MEG experiment: predictions and measurements

The MEG experiment makes use of one of the world’s most intense low energy muon beams, in order to search for the lepton flavour violating process μ+→e+γ . We determined the residual beam polarization at the thin stopping target, by measuring the asymmetry of the angular distribution of Michel decay positrons as a function of energy. The initial muon beam polarization at the production is predicted to be Pμ=−1Pμ=−1 by the Standard Model (SM) with massless neutrinos.

Ferromagnetic Quantum Critical Point Avoided by the Appearance of Another Magnetic Phase in LaCrGe3 under Pressure

The temperature-pressure phase diagram of the ferromagnet LaCrGe3 is determined for the first time from a combination of magnetization, muon-spin-rotation, and electrical resistivity measurements. The ferromagnetic phase is suppressed near 2.1 GPa, but quantum criticality is avoided by the appearance of a magnetic phase, likely modulated, AFMQ.

Momentum-Resolved Electronic Structure of the High-Tc Superconductor Parent Compound BaBiO3

We investigate the band structure of BaBiO3, an insulating parent compound of doped high-Tc superconductors, using in situ angle-resolved photoemission spectroscopy on thin films. The data compare favorably overall with density functional theory calculations within the local density approximation, demonstrating that electron correlations are weak. The bands exhibit Brillouin zone folding consistent with known BiO6 breathing distortions.

DSC00750.jpg

LUC at the Top of Europe

This years excursion took the members of the Laboratory of Environmental Chemistry (LUC) up to 3600 m altitude where we visited the high-alpine research station. We enjoyed Heinz Gäggeler, president of the Swiss Commission of the high-alpine research station Jungfraujoch, giving us a tour through the station and a live demonstration of ice core drilling.

optofluidic.jpg

Therapeutic drug monitoring in sub-nanoliter volumes

A promising system for painless and minimally-invasive therapeutic drug monitoring has been demonstrated. The proposed device combines biofunctionalized hollow microneedles with an optofluidic system to measure drug concentrations in volumes as small as 0.6 nL.

Co magnetic moment as a function of applied electric field

Magnetoelectroelastic control of magnetism

X-ray magnetic circular dichroism at the Co L3,2 edges measured at the X-Treme beamline, SLS and at the Advanced Light Source, evidence that three distinct electric field driven remanent magnetization states can be set in the Co film at room temperature. Ab initio density functional theory calculations unravel the relative contributions of both strain and charge to the observed magnetic anisotropy changes illustrating magnetoelectroelastic coupling at artificial multiferroic interfaces.

Controlling Quantum States Atom by Atom

A method to precisely alter the quantum mechanical states of electrons within an array of quantum boxes has been developped by an international consortium also including PSI. The method can be used to investigate the interactions between various types of atoms and electrons, which is essential for future quantum technologies.